| 李春霞,贾美林,郭少红,贾晶春.金属纳米簇在CO2光催化还原中的研究进展[J].分子催化,2023,37(6):614-624 |
| 金属纳米簇在CO2光催化还原中的研究进展 |
| Research Progress of Carbon Dioxide Photoreduction Based on the Catalyst of Metal Nanoclusters |
| 投稿时间：2023-07-27 修订日期：2023-09-16 |
| DOI：10.16084/j.issn1001-3555.2023.06.009 |
| 中文关键词: 金属纳米簇 光催化 CO2还原 |
| 英文关键词:metal nanoclusters photocatalysis CO2 reduction |
| 基金项目:内蒙古自然科学基金 (项目编号: 2021BS02019); 内蒙古师范大学科研启动基金 (No. 2020YJRC012); 内蒙古师范大学基本科研业务费专项资金资助(项目编号: 2022JBXC015); 内蒙古师范大学研究生科研创新基金资助项目(项目编号: CXJJS22114) |
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| 中文摘要: |
| 以清洁、储量丰富的太阳光作为能量来源, 将二氧化碳 (CO2) 光催化还原为高附加值的化学产品是缓解当前环境和能源问题的主要方法之一. 然而, CO2在常温常压下非常的稳定, 因此需要设计并构筑高效光催化剂来捕捉和转化CO2以提高光催化CO2还原的效率. 在众多研究的光催化剂中, 金属纳米簇因其具有独特的结构特点、优异的物理和化学性质在光催化CO2还原领域得到了广泛的应用. 接下来对金属纳米簇进行了分类, 将金属纳米簇分为贵金属纳米簇和非贵金属纳米簇. 对贵金属纳米簇和非贵金属在光催化CO2还原的特点和应用做出了简单介绍与总结. |
| 英文摘要: |
| The massive burning of fossil fuels not only causes an energy crisis, but also emits carbon dioxide (CO2) that warms the climate. Using clean and abundant sunlight as an energy source, photocatalytic reduction of CO2 into high value-added chemical products is one of the main ways to alleviate current environmental and energy problems. However, CO2 is very stable at room temperature and pressure, so it is necessary to design and build efficient photocatalysts to capture and transform CO2 to achieve the purpose of efficient photocatalytic CO2 reduction. Among the photocatalysts studied, metal nanoclusters have been widely used in the field of photocatalytic CO2 reduction because of their unique structural characteristics and excellent physical and chemical properties. Based on this, we first classify metal nanoclusters into noble metal nanoclusters and non-precious metal nanoclusters. Then, the research progress of noble metal and non-noble metal nanoclusters in photocatalytic CO2 reduction was summarized. This paper summarizes the research progress in this field in a timely and comprehensive manner and provides new ideas for future research. |
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